Suppression of antiferromagnetic order by strain-enhanced frustration in honeycomb cobaltate

Authors: Gye-Hyeon Kim, Miju Park, Subhasis Samanta, Uksam Choi, Baekjune Kang, Uihyeon Seo, GwangCheol Ji, Seunghyeon Noh, Deok-Yong Cho, Jung-Woo Yoo, Jong Mok Ok, Heung-Sik Kim, Changhee Sohn

Published: 2024-07-05

DOI: 10.1126/sciadv.adn8694

Source: Full article


Abstract

Layered honeycomb cobaltates are predicted as promising for realizing the Kitaev quantum spin liquid, a many-body quantum entangled ground state characterized by fractional excitations. However, they exhibit antiferromagnetic ordering at low temperatures, hindering the expected quantum state. We demonstrate that controlling the trigonal distortion of CoO